If this engine has not had a valve adjustment and has been neglected by the prior owner/s, you may have to do a couple more.
Do the first adjustment, put a 100 miles on it. do another etc...
If it has not been done in a long while. carbon builds up in the seats, and as the valves rotate, the carbon wears off and throws out the adj.
They are suppose to be done once a yr or every 15K miles.
Here is the list of DIY, it`s in the OM617 section.
PeachPartsWiki: Do It Yourself Articles - Mercedes Vehicles
Here is a good thread if you really want to get into replacing the chain and other related parts.
http://www.peachparts.com/shopforum/diesel-discussion/305365-9-degrees-chain-stretch.html